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Publication:
Tuning the selectivity of single-site supported metal catalysts with ionic liquids

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Fang, Chia-Yu

Hoffman, Adam S.

Bare, Simon R.

Gates, Bruce C.

Date

2017

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Journal Article

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Abstract

1,3-Dialkylimidazolium ionic liquid coatings act as electron donors, increasing the selectivity for partial hydrogenation of 1,3-butadiene catalyzed by iridium complexes supported on high-surface-area gamma-Al2O3. High-energy-resolution fluorescence detection X-ray absorption near-edge structure (HERFD XANES) measurements quantify the electron donation and are correlated with the catalytic activity and selectivity. The results demonstrate broad opportunities to tune electronic environments and catalytic properties of atomically dispersed supported metal catalysts.

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American Chemical Society (ACS)

Subject

Chemistry , Physical

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Acs Catalysis

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DOI

10.1021/acscatal.7b02429

URI

https://doi.org/10.1021/acscatal.7b02429
 https://hdl.handle.net/20.500.14288/11061

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