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Role of chain symmetry and hydrogen bonding in segmented copolymers with monodisperse hard segments

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Sheth, JP
Klinedinst, DB
Wilkes, GL
Iskender, Y

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Abstract

Thermoplastic segmented polyurethane and polyurea copolymers whose monodisperse hard segments are based on only a single diisocyanate molecule are discussed. The solid-state structure-property behavior of these materials demonstrates that a proper selection of the level of symmetry and/or cohesiveness of the hard microdomains may allow elimination of the traditional requirement of chain extension to obtain melt processable segmented urethanes, and more specifically, urea copolymers with useful structural properties.

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Elsevier Sci Ltd

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Polymers, Polymerization

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Polymer

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10.1016/j.polymer.2005.04.041

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